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Abstract

A method for producing carbon negative cementitious materials utilizing a carbon mineralization-based direct-air capture process. The method comprises a mineralization step wherein a mineral feedstock is contacted with an aqueous carbonate solution at a high initial pH to form a carbonated feedstock containing reactive silica, along with an alkaline solution containing dissolved aluminum. The resulting alkaline solution is then contacted with gaseous carbon dioxide to form a carbonate solution that can be recycled for use in the mineralization step. The dissolved aluminum in the alkaline solution precipitates during carbon dioxide capture and is subsequently redissolved in a hydroxide solution to form alumina. The alumina can be combined with the carbonated feedstock to create geopolymer concrete.

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First Claim